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Interfacing Silicon-Based Quantum Dots with Proteins for Biological and Sensing Applications
DownloadFall 2020
This dissertation presents the preparation of functional bioinorganic hybrids from silicon-based quantum dots (SiQDs) and enzymes and the use of SiQDs and green fluorescent protein as ratiometric photoluminescent sensors for nerve agents. Chapter 2 discusses the preparation of water-soluble...
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Investigation of the Adsorption of Model and Oil Sands Process-Affected Water Naphthenic Acids on Graphite
DownloadSpring 2015
Naphthenic acids (NAs) are constituents of bitumen in the oil sands deposits in northern Alberta, Canada. The extraction process of bitumen creates an enormous amount of wastewater called oil sands process affected waters (OSPW). This OSPW contains elevated concentrations of NAs, and other...
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Fall 2010
This thesis describes the fabrication and characterization of integrated hollow Bragg waveguides fabricated by controlled thin film buckling. Hollow waveguides based on two different set of materials were studied. In the first case, thermal tuning of air-core dimensions was studied using...
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Nanolithography on H:Si(100)-(2 x 1) using combined Scanning Tunneling Microscopy and Field Ion Microscopy techniques
DownloadFall 2011
This thesis reports on the combined techniques of ultra-high vacuum scanning tunneling microscopy (UHV-STM) and field ion microscopy (FIM). The apex structure of STM scanning tips correlates with their ability to yield highly-resolved images and to perform accurate hydrogen desorption on...
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Observing and Manipulating Single Electrons Confined to Silicon Dangling Bond Ensembles with Non-Contact Atomic Force Microscopy
DownloadFall 2018
Non-contact atomic force microscopy (nc-AFM) is capable of inducing and resolving single-electron charge transitions of surface adsorbates. Here, these techniques are extended by studying the charge configurations of dangling bond (DB) ensembles on the hydrogen-terminated silicon surface. nc-AFM...
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Probing Surface Heterogeneity, Electrochemical Properties and Bubble-Solid Interaction Mechanisms of Sulfide Minerals in Flotation
DownloadSpring 2017
The colloidal stability governed by various surface interactions including van der Waals (VDW) interaction, electrical double layer (EDL) interaction, hydrophobic interaction, and some other interactions, plays an important role in a wide range of natural phenomena and engineering applications....
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Fall 2014
This thesis is focused on the Si-based anode materials for lithium-ion batteries (LIBs) as well as biomass-derived carbons for LIBs and sodium-ion batteries (NIBs). In our first attempt we investigated the effect of the support growth substrate as well as of aluminum coating layers on the...
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Spring 2015
This thesis is focused on the silicon-based anode materials for lithium-ion batteries (LIBs) as well as germanium-based electrode materials for sodium-ion batteries (NIBs). In our first attempt we studied electrochemical cycling stability and degradation mechanisms of silicon nanowires (SiNWs)...
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Spring 2017
We present the characterization of close-spaced linear dangling bond structures, or dangling bond chains, two to seven dangling bonds long, on a hydrogen terminated silicon (100)-2x1 surface using a scan- ning tunnelling microscope. Constant height differential conductance maps reveal their local...
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Fall 2015
Dangling Bonds (DBs) on the silicon surface exist when a silicon atom lacks a bonding partner, resulting in a localized orbital which is not involved in any chemical bonds. On the hydrogen-terminated Si(100) surface, such DBs introduce a mid-gap state. DBs can be created on this surface by the...