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A general route to 1,3'-bipyrroles, conversion of cyclohexenone-type systems into phenols and synthetic studies on Coleophomone B
DownloadFall 2016
Chapter 1 describes a general route for making 1,3'-bipyrroles. This work involves intermolecular conjugate displacement using a special Michael acceptor developed in this laboratory. This method is general and enables the construction of highly substituted 1,3'-bipyrroles. The route was first...
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Fall 2017
Chapter 1 describes the total synthesis of (+)-ipalbidine. The indolizidine core structure was formed by use of an unusual 6-exo-trigonal radical cyclization as a key step. I started from the chiral pool using L-proline and obtained ipalbidine with an ee of >99.6%. Chapter 2 describes synthetic...