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Morphology control and localized surface plasmon resonance in glancing angle deposited films Open Access

Descriptions

Other title
Subject/Keyword
thin film
phi-sweep
biosensing
localized surface plasmon resonance
glancing angle deposition
Type of item
Thesis
Degree grantor
University of Alberta
Author or creator
Gish, Douglas
Supervisor and department
Brett, Michael (Electrical and Computer Engineering)
Examining committee member and department
Sit, Jeremy (Electrical and Computer Engineering)
McDermott, Mark (Chemistry)
Brett, Michael (Electrical and Computer Engineering)
Department
Department of Electrical and Computer Engineering
Specialization

Date accepted
2010-08-12T14:45:24Z
Graduation date
2010-11
Degree
Master of Science
Degree level
Master's
Abstract
This research investigates an extension of the glancing angle deposition (GLAD) technique and a biosensing application of films produced by GLAD. The extension to GLAD, called phi-sweep (PS), improves column isolation compared to films grown by traditional GLAD (TG) as well as modifies the column tilt angle, β, of the slanted columns according to tan(β_{PS}) = tan(β_{TG}) cos(γ), where γ is the sweep angle. The biosensing application makes use of localized surface plasmon resonance in noble metal GLAD films functionalized with rabbit immunoglobulin G (rIgG) to detect binding of anti-rabbit immunoglobulin G (anti-rIgG) to the films' surface. The extinction peak red-shifts a distance dependent on the concentration of anti-rIgG solution in a manner described by the Langmuir isotherm with a saturation value, Δλ_{max}, of 29.4 ± 0.7 nm and a surface confined thermodynamic binding constant, Kₐ, of (2.7 ± 0.3)×10⁶ M⁻¹.
Language
English
Rights
Permission is hereby granted to the University of Alberta Libraries to reproduce single copies of this thesis and to lend or sell such copies for private, scholarly or scientific research purposes only. Where the thesis is converted to, or otherwise made available in digital form, the University of Alberta will advise potential users of the thesis of these terms. The author reserves all other publication and other rights in association with the copyright in the thesis and, except as herein before provided, neither the thesis nor any substantial portion thereof may be printed or otherwise reproduced in any material form whatsoever without the author's prior written permission.
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File format: pdf (Portable Document Format)
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File size: 103625182
Last modified: 2015:10:12 18:39:07-06:00
Filename: Gish_Douglas_Fall 2010.pdf
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File title: Preface
File author: Douglas Gish
Page count: 92
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